Abstract
Baseline correction is a vital part of spectral preprocessing, especially for Raman spectra. Iterative polynomial fitting is an easy but less accurate way to find baselines compared to other methods such as wavelet transform and penalized least squares (PLS) methods. The polynomial fitting methods can also get distorted results in certain conditions. In this paper, a neural network model for detecting the trend of the baseline was proposed to improve the correction accuracy of the fitting methods. The model selects the function basis according to the baseline trend instead of using a fixed polynomial function to match the baseline for a more precise fit. We also propose a way to generate simulation data, these data can be used to train the neural network model. The model provides reliable results for real spectral data with noise. Our method provides a new idea to correct the baseline with a strange shape. In addition, we examine the limitations of conventional iterative polynomial fitting, adaptive iteratively reweighted PLS and explain why our approach surpasses these methods.
This is a visual representation of the abstract.
Keywords
Get full access to this article
View all access options for this article.
References
Supplementary Material
Please find the following supplemental material available below.
For Open Access articles published under a Creative Commons License, all supplemental material carries the same license as the article it is associated with.
For non-Open Access articles published, all supplemental material carries a non-exclusive license, and permission requests for re-use of supplemental material or any part of supplemental material shall be sent directly to the copyright owner as specified in the copyright notice associated with the article.
